MozartV1, PascalFrancis, Corpus, bibRecord, 000112

Contribution of isoprene to chemical budgets : A model tracer study with the NCAR CTM MOZART-4

Identifieur interne : 000112 ( PascalFrancis/Corpus ); précédent : 000111; suivant : 000113

Contribution of isoprene to chemical budgets : A model tracer study with the NCAR CTM MOZART-4

Auteurs : G. G. Pfister ; L. K. Emmons ; P. G. Hess ; J.-F. Lamarque ; J. J. Orlando ; S. Walters ; A. Guenther ; P. I. Palmer ; P. J. Lawrence

Source :

Journal of geophysical research [ 0148-0227 ] ; 2008.

RBID : Pascal:08-0208587

Descripteurs français

Pascal (Inist)
- Isoprène, Modèle, Traceur, Analyse sensibilité, Monde, Transport, Occupation sol, Troposphère, Ozone, Gaz, Aérosol, Trajectoire, Carbone, Oxydation, Monoxyde carbone, Monoxyde de carbone, Formaldéhyde, Peracétique acide nitrate, Pan, Echelle planétaire, Concentration, Composé trace, Variabilité.

English descriptors

KwdEn :
- Carbon monoxide, Formaldehyde, Isoprene, Pan, Peroxyacetyl nitrate, Planetary scale, Trace compound, aerosols, carbon, carbon monoxide, concentration, gases, global, land cover, models, oxidation, ozone, sensitivity analysis, tracers, trajectory, transport, troposphere, variability.

Abstract

[1] We present a study of the sensitivity of isoprene emission calculations in a global chemistry transport model (CTM) to input land cover characteristics and analyze the impacts of changes in isoprene on the tropospheric budgets of atmospheric key species. The CTM Model for Ozone and Related Chemical Species, version 4 (MOZART-4) includes the online calculation of isoprene emissions based on the Model of Emissions of Gases and Aerosols from Nature (MEGAN), which is driven by three different land parameter inputs. We also included a tagging scheme in the CTM, which keeps track of the production of carbon containing species from isoprene oxidation. It is found that the amount of tropospheric carbon monoxide (CO), formaldehyde (HCHO) and peroxyacetylnitrate (PAN) explained by isoprene oxidation ranges from 9-16%, 15-27%, and 22-32%, depending on the isoprene emissions scenario. Changes in the global tropospheric burden with different land cover inputs can reach up to 10% for CO, 15% for HCHO, and 20% for PAN. Changes for ozone are small on a global scale, but regionally differences are as large as 3DU in the tropospheric column and as large as 5 ppbv in the surface concentrations. Our results demonstrate that a careful integration of isoprene emissions and chemistry in CTMs is very important for simulating the budgets of a number of atmospheric trace gases. We further demonstrate that the model tagging scheme has the capability of improving conventional methods of constraining isoprene emissions from space-borne HCHO column observations, especially in regions where a considerable part of the variability in the HCHO column is not related to isoprene.

Notice en format standard (ISO 2709)

Pour connaître la documentation sur le format Inist Standard.

A01	`01`	`1`		`@0 0148-0227`
A03		`1`		`@0 J. geophys. res.`
A05				`@2 113`
A06				`@2 D5`
A08	`01`	`1`	`ENG`	`@1 Contribution of isoprene to chemical budgets : A model tracer study with the NCAR CTM MOZART-4`
A11	`01`	`1`		`@1 PFISTER (G. G.)`
A11	`02`	`1`		`@1 EMMONS (L. K.)`
A11	`03`	`1`		`@1 HESS (P. G.)`
A11	`04`	`1`		`@1 LAMARQUE (J.-F.)`
A11	`05`	`1`		`@1 ORLANDO (J. J.)`
A11	`06`	`1`		`@1 WALTERS (S.)`
A11	`07`	`1`		`@1 GUENTHER (A.)`
A11	`08`	`1`		`@1 PALMER (P. I.)`
A11	`09`	`1`		`@1 LAWRENCE (P. J.)`
A14	`01`			`@1 National Center for Atmospheric Research @2 Boulder, Colorado @3 USA @Z 1 aut. @Z 2 aut. @Z 3 aut. @Z 4 aut. @Z 5 aut. @Z 6 aut. @Z 7 aut.`
A14	`02`			`@1 School of GeoSciences, University of Edinburgh @2 Edinburgh @3 GBR @Z 8 aut.`
A14	`03`			`@1 Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado @2 Boulder, Colorado @3 USA @Z 9 aut.`
A20				`@2 D05308.1-D05308.21`
A21				`@1 2008`
A23	`01`			`@0 ENG`
A43	`01`			`@1 INIST @2 3144 @5 354000183022170370`
A44				`@0 0000 @1 © 2008 INIST-CNRS. All rights reserved.`
A45				`@0 1 p.1/2`
A47	`01`	`1`		`@0 08-0208587`
A60				`@1 P`
A61				`@0 A`
A64	`01`	`1`		`@0 Journal of geophysical research`
A66	`01`			`@0 USA`
C01	`01`		`ENG`	@0 [1] We present a study of the sensitivity of isoprene emission calculations in a global chemistry transport model (CTM) to input land cover characteristics and analyze the impacts of changes in isoprene on the tropospheric budgets of atmospheric key species. The CTM Model for Ozone and Related Chemical Species, version 4 (MOZART-4) includes the online calculation of isoprene emissions based on the Model of Emissions of Gases and Aerosols from Nature (MEGAN), which is driven by three different land parameter inputs. We also included a tagging scheme in the CTM, which keeps track of the production of carbon containing species from isoprene oxidation. It is found that the amount of tropospheric carbon monoxide (CO), formaldehyde (HCHO) and peroxyacetylnitrate (PAN) explained by isoprene oxidation ranges from 9-16%, 15-27%, and 22-32%, depending on the isoprene emissions scenario. Changes in the global tropospheric burden with different land cover inputs can reach up to 10% for CO, 15% for HCHO, and 20% for PAN. Changes for ozone are small on a global scale, but regionally differences are as large as 3DU in the tropospheric column and as large as 5 ppbv in the surface concentrations. Our results demonstrate that a careful integration of isoprene emissions and chemistry in CTMs is very important for simulating the budgets of a number of atmospheric trace gases. We further demonstrate that the model tagging scheme has the capability of improving conventional methods of constraining isoprene emissions from space-borne HCHO column observations, especially in regions where a considerable part of the variability in the HCHO column is not related to isoprene.
C02	`01`	`3`		`@0 001E`
C02	`02`	`2`		`@0 001E01`
C02	`03`	`2`		`@0 220`
C03	`01`	`X`	`FRE`	`@0 Isoprène @2 NK @5 01`
C03	`01`	`X`	`ENG`	`@0 Isoprene @2 NK @5 01`
C03	`01`	`X`	`SPA`	`@0 Isopreno @2 NK @5 01`
C03	`02`	`2`	`FRE`	`@0 Modèle @5 02`
C03	`02`	`2`	`ENG`	`@0 models @5 02`
C03	`02`	`2`	`SPA`	`@0 Modelo @5 02`
C03	`03`	`2`	`FRE`	`@0 Traceur @5 03`
C03	`03`	`2`	`ENG`	`@0 tracers @5 03`
C03	`03`	`2`	`SPA`	`@0 Trazador @5 03`
C03	`04`	`2`	`FRE`	`@0 Analyse sensibilité @5 04`
C03	`04`	`2`	`ENG`	`@0 sensitivity analysis @5 04`
C03	`05`	`2`	`FRE`	`@0 Monde @5 05`
C03	`05`	`2`	`ENG`	`@0 global @5 05`
C03	`05`	`2`	`SPA`	`@0 Mundo @5 05`
C03	`06`	`2`	`FRE`	`@0 Transport @5 06`
C03	`06`	`2`	`ENG`	`@0 transport @5 06`
C03	`06`	`2`	`SPA`	`@0 Transporte @5 06`
C03	`07`	`2`	`FRE`	`@0 Occupation sol @5 07`
C03	`07`	`2`	`ENG`	`@0 land cover @5 07`
C03	`08`	`2`	`FRE`	`@0 Troposphère @5 08`
C03	`08`	`2`	`ENG`	`@0 troposphere @5 08`
C03	`09`	`2`	`FRE`	`@0 Ozone @5 09`
C03	`09`	`2`	`ENG`	`@0 ozone @5 09`
C03	`09`	`2`	`SPA`	`@0 Ozono @5 09`
C03	`10`	`2`	`FRE`	`@0 Gaz @5 10`
C03	`10`	`2`	`ENG`	`@0 gases @5 10`
C03	`10`	`2`	`SPA`	`@0 Gas @5 10`
C03	`11`	`2`	`FRE`	`@0 Aérosol @5 11`
C03	`11`	`2`	`ENG`	`@0 aerosols @5 11`
C03	`11`	`2`	`SPA`	`@0 Aerosol @5 11`
C03	`12`	`2`	`FRE`	`@0 Trajectoire @5 12`
C03	`12`	`2`	`ENG`	`@0 trajectory @5 12`
C03	`13`	`2`	`FRE`	`@0 Carbone @5 13`
C03	`13`	`2`	`ENG`	`@0 carbon @5 13`
C03	`13`	`2`	`SPA`	`@0 Carbono @5 13`
C03	`14`	`2`	`FRE`	`@0 Oxydation @5 14`
C03	`14`	`2`	`ENG`	`@0 oxidation @5 14`
C03	`14`	`2`	`SPA`	`@0 Oxidación @5 14`
C03	`15`	`2`	`FRE`	`@0 Monoxyde carbone @5 15`
C03	`15`	`2`	`ENG`	`@0 carbon monoxide @5 15`
C03	`16`	`X`	`FRE`	`@0 Monoxyde de carbone @2 NK @2 FX @5 16`
C03	`16`	`X`	`ENG`	`@0 Carbon monoxide @2 NK @2 FX @5 16`
C03	`16`	`X`	`SPA`	`@0 Carbono monóxido @2 NK @2 FX @5 16`
C03	`17`	`X`	`FRE`	`@0 Formaldéhyde @2 NK @2 FX @5 17`
C03	`17`	`X`	`ENG`	`@0 Formaldehyde @2 NK @2 FX @5 17`
C03	`17`	`X`	`SPA`	`@0 Formaldehído @2 NK @2 FX @5 17`
C03	`18`	`3`	`FRE`	`@0 Peracétique acide nitrate @2 NK @5 18`
C03	`18`	`3`	`ENG`	`@0 Peroxyacetyl nitrate @2 NK @5 18`
C03	`19`	`X`	`FRE`	`@0 Pan @2 NO @5 19`
C03	`19`	`X`	`ENG`	`@0 Pan @2 NO @5 19`
C03	`19`	`X`	`SPA`	`@0 Pan @2 NO @5 19`
C03	`20`	`X`	`FRE`	`@0 Echelle planétaire @5 20`
C03	`20`	`X`	`ENG`	`@0 Planetary scale @5 20`
C03	`20`	`X`	`SPA`	`@0 Escala planetaria @5 20`
C03	`21`	`2`	`FRE`	`@0 Concentration @5 21`
C03	`21`	`2`	`ENG`	`@0 concentration @5 21`
C03	`21`	`2`	`SPA`	`@0 Concentración @5 21`
C03	`22`	`X`	`FRE`	`@0 Composé trace @5 22`
C03	`22`	`X`	`ENG`	`@0 Trace compound @5 22`
C03	`22`	`X`	`SPA`	`@0 Compuesto huella @5 22`
C03	`23`	`2`	`FRE`	`@0 Variabilité @5 23`
C03	`23`	`2`	`ENG`	`@0 variability @5 23`
N21				`@1 133`
N44	`01`			`@1 OTO`
N82				`@1 OTO`

Format Inist (serveur)

NO :	PASCAL 08-0208587 INIST
ET :	Contribution of isoprene to chemical budgets : A model tracer study with the NCAR CTM MOZART-4
AU :	PFISTER (G. G.); EMMONS (L. K.); HESS (P. G.); LAMARQUE (J.-F.); ORLANDO (J. J.); WALTERS (S.); GUENTHER (A.); PALMER (P. I.); LAWRENCE (P. J.)
AF :	National Center for Atmospheric Research/Boulder, Colorado/Etats-Unis (1 aut., 2 aut., 3 aut., 4 aut., 5 aut., 6 aut., 7 aut.); School of GeoSciences, University of Edinburgh/Edinburgh/Royaume-Uni (8 aut.); Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado/Boulder, Colorado/Etats-Unis (9 aut.)
DT :	Publication en série; Niveau analytique
SO :	Journal of geophysical research; ISSN 0148-0227; Etats-Unis; Da. 2008; Vol. 113; No. D5; D05308.1-D05308.21; Bibl. 1 p.1/2
LA :	Anglais
EA :	[1] We present a study of the sensitivity of isoprene emission calculations in a global chemistry transport model (CTM) to input land cover characteristics and analyze the impacts of changes in isoprene on the tropospheric budgets of atmospheric key species. The CTM Model for Ozone and Related Chemical Species, version 4 (MOZART-4) includes the online calculation of isoprene emissions based on the Model of Emissions of Gases and Aerosols from Nature (MEGAN), which is driven by three different land parameter inputs. We also included a tagging scheme in the CTM, which keeps track of the production of carbon containing species from isoprene oxidation. It is found that the amount of tropospheric carbon monoxide (CO), formaldehyde (HCHO) and peroxyacetylnitrate (PAN) explained by isoprene oxidation ranges from 9-16%, 15-27%, and 22-32%, depending on the isoprene emissions scenario. Changes in the global tropospheric burden with different land cover inputs can reach up to 10% for CO, 15% for HCHO, and 20% for PAN. Changes for ozone are small on a global scale, but regionally differences are as large as 3DU in the tropospheric column and as large as 5 ppbv in the surface concentrations. Our results demonstrate that a careful integration of isoprene emissions and chemistry in CTMs is very important for simulating the budgets of a number of atmospheric trace gases. We further demonstrate that the model tagging scheme has the capability of improving conventional methods of constraining isoprene emissions from space-borne HCHO column observations, especially in regions where a considerable part of the variability in the HCHO column is not related to isoprene.
CC :	001E; 001E01; 220
FD :	Isoprène; Modèle; Traceur; Analyse sensibilité; Monde; Transport; Occupation sol; Troposphère; Ozone; Gaz; Aérosol; Trajectoire; Carbone; Oxydation; Monoxyde carbone; Monoxyde de carbone; Formaldéhyde; Peracétique acide nitrate; Pan; Echelle planétaire; Concentration; Composé trace; Variabilité
ED :	Isoprene; models; tracers; sensitivity analysis; global; transport; land cover; troposphere; ozone; gases; aerosols; trajectory; carbon; oxidation; carbon monoxide; Carbon monoxide; Formaldehyde; Peroxyacetyl nitrate; Pan; Planetary scale; concentration; Trace compound; variability
SD :	Isopreno; Modelo; Trazador; Mundo; Transporte; Ozono; Gas; Aerosol; Carbono; Oxidación; Carbono monóxido; Formaldehído; Pan; Escala planetaria; Concentración; Compuesto huella
LO :	INIST-3144.354000183022170370
ID :	08-0208587

Links to Exploration step

Pascal:08-0208587

Le document en format XML

<record><TEI><teiHeader><fileDesc><titleStmt><title xml:lang="en" level="a">Contribution of isoprene to chemical budgets : A model tracer study with the NCAR CTM MOZART-4</title>
<author><name sortKey="Pfister, G G" sort="Pfister, G G" uniqKey="Pfister G" first="G. G." last="Pfister">G. G. Pfister</name>
<affiliation><inist:fA14 i1="01"><s1>National Center for Atmospheric Research</s1>
<s2>Boulder, Colorado</s2>
<s3>USA</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
<sZ>3 aut.</sZ>
<sZ>4 aut.</sZ>
<sZ>5 aut.</sZ>
<sZ>6 aut.</sZ>
<sZ>7 aut.</sZ>
</inist:fA14>
</affiliation>
</author>
<author><name sortKey="Emmons, L K" sort="Emmons, L K" uniqKey="Emmons L" first="L. K." last="Emmons">L. K. Emmons</name>
<affiliation><inist:fA14 i1="01"><s1>National Center for Atmospheric Research</s1>
<s2>Boulder, Colorado</s2>
<s3>USA</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
<sZ>3 aut.</sZ>
<sZ>4 aut.</sZ>
<sZ>5 aut.</sZ>
<sZ>6 aut.</sZ>
<sZ>7 aut.</sZ>
</inist:fA14>
</affiliation>
</author>
<author><name sortKey="Hess, P G" sort="Hess, P G" uniqKey="Hess P" first="P. G." last="Hess">P. G. Hess</name>
<affiliation><inist:fA14 i1="01"><s1>National Center for Atmospheric Research</s1>
<s2>Boulder, Colorado</s2>
<s3>USA</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
<sZ>3 aut.</sZ>
<sZ>4 aut.</sZ>
<sZ>5 aut.</sZ>
<sZ>6 aut.</sZ>
<sZ>7 aut.</sZ>
</inist:fA14>
</affiliation>
</author>
<author><name sortKey="Lamarque, J F" sort="Lamarque, J F" uniqKey="Lamarque J" first="J.-F." last="Lamarque">J.-F. Lamarque</name>
<affiliation><inist:fA14 i1="01"><s1>National Center for Atmospheric Research</s1>
<s2>Boulder, Colorado</s2>
<s3>USA</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
<sZ>3 aut.</sZ>
<sZ>4 aut.</sZ>
<sZ>5 aut.</sZ>
<sZ>6 aut.</sZ>
<sZ>7 aut.</sZ>
</inist:fA14>
</affiliation>
</author>
<author><name sortKey="Orlando, J J" sort="Orlando, J J" uniqKey="Orlando J" first="J. J." last="Orlando">J. J. Orlando</name>
<affiliation><inist:fA14 i1="01"><s1>National Center for Atmospheric Research</s1>
<s2>Boulder, Colorado</s2>
<s3>USA</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
<sZ>3 aut.</sZ>
<sZ>4 aut.</sZ>
<sZ>5 aut.</sZ>
<sZ>6 aut.</sZ>
<sZ>7 aut.</sZ>
</inist:fA14>
</affiliation>
</author>
<author><name sortKey="Walters, S" sort="Walters, S" uniqKey="Walters S" first="S." last="Walters">S. Walters</name>
<affiliation><inist:fA14 i1="01"><s1>National Center for Atmospheric Research</s1>
<s2>Boulder, Colorado</s2>
<s3>USA</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
<sZ>3 aut.</sZ>
<sZ>4 aut.</sZ>
<sZ>5 aut.</sZ>
<sZ>6 aut.</sZ>
<sZ>7 aut.</sZ>
</inist:fA14>
</affiliation>
</author>
<author><name sortKey="Guenther, A" sort="Guenther, A" uniqKey="Guenther A" first="A." last="Guenther">A. Guenther</name>
<affiliation><inist:fA14 i1="01"><s1>National Center for Atmospheric Research</s1>
<s2>Boulder, Colorado</s2>
<s3>USA</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
<sZ>3 aut.</sZ>
<sZ>4 aut.</sZ>
<sZ>5 aut.</sZ>
<sZ>6 aut.</sZ>
<sZ>7 aut.</sZ>
</inist:fA14>
</affiliation>
</author>
<author><name sortKey="Palmer, P I" sort="Palmer, P I" uniqKey="Palmer P" first="P. I." last="Palmer">P. I. Palmer</name>
<affiliation><inist:fA14 i1="02"><s1>School of GeoSciences, University of Edinburgh</s1>
<s2>Edinburgh</s2>
<s3>GBR</s3>
<sZ>8 aut.</sZ>
</inist:fA14>
</affiliation>
</author>
<author><name sortKey="Lawrence, P J" sort="Lawrence, P J" uniqKey="Lawrence P" first="P. J." last="Lawrence">P. J. Lawrence</name>
<affiliation><inist:fA14 i1="03"><s1>Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado</s1>
<s2>Boulder, Colorado</s2>
<s3>USA</s3>
<sZ>9 aut.</sZ>
</inist:fA14>
</affiliation>
</author>
</titleStmt>
<publicationStmt><idno type="wicri:source">INIST</idno>
<idno type="inist">08-0208587</idno>
<date when="2008">2008</date>
<idno type="stanalyst">PASCAL 08-0208587 INIST</idno>
<idno type="RBID">Pascal:08-0208587</idno>
<idno type="wicri:Area/PascalFrancis/Corpus">000112</idno>
</publicationStmt>
<sourceDesc><biblStruct><analytic><title xml:lang="en" level="a">Contribution of isoprene to chemical budgets : A model tracer study with the NCAR CTM MOZART-4</title>
<author><name sortKey="Pfister, G G" sort="Pfister, G G" uniqKey="Pfister G" first="G. G." last="Pfister">G. G. Pfister</name>
<affiliation><inist:fA14 i1="01"><s1>National Center for Atmospheric Research</s1>
<s2>Boulder, Colorado</s2>
<s3>USA</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
<sZ>3 aut.</sZ>
<sZ>4 aut.</sZ>
<sZ>5 aut.</sZ>
<sZ>6 aut.</sZ>
<sZ>7 aut.</sZ>
</inist:fA14>
</affiliation>
</author>
<author><name sortKey="Emmons, L K" sort="Emmons, L K" uniqKey="Emmons L" first="L. K." last="Emmons">L. K. Emmons</name>
<affiliation><inist:fA14 i1="01"><s1>National Center for Atmospheric Research</s1>
<s2>Boulder, Colorado</s2>
<s3>USA</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
<sZ>3 aut.</sZ>
<sZ>4 aut.</sZ>
<sZ>5 aut.</sZ>
<sZ>6 aut.</sZ>
<sZ>7 aut.</sZ>
</inist:fA14>
</affiliation>
</author>
<author><name sortKey="Hess, P G" sort="Hess, P G" uniqKey="Hess P" first="P. G." last="Hess">P. G. Hess</name>
<affiliation><inist:fA14 i1="01"><s1>National Center for Atmospheric Research</s1>
<s2>Boulder, Colorado</s2>
<s3>USA</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
<sZ>3 aut.</sZ>
<sZ>4 aut.</sZ>
<sZ>5 aut.</sZ>
<sZ>6 aut.</sZ>
<sZ>7 aut.</sZ>
</inist:fA14>
</affiliation>
</author>
<author><name sortKey="Lamarque, J F" sort="Lamarque, J F" uniqKey="Lamarque J" first="J.-F." last="Lamarque">J.-F. Lamarque</name>
<affiliation><inist:fA14 i1="01"><s1>National Center for Atmospheric Research</s1>
<s2>Boulder, Colorado</s2>
<s3>USA</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
<sZ>3 aut.</sZ>
<sZ>4 aut.</sZ>
<sZ>5 aut.</sZ>
<sZ>6 aut.</sZ>
<sZ>7 aut.</sZ>
</inist:fA14>
</affiliation>
</author>
<author><name sortKey="Orlando, J J" sort="Orlando, J J" uniqKey="Orlando J" first="J. J." last="Orlando">J. J. Orlando</name>
<affiliation><inist:fA14 i1="01"><s1>National Center for Atmospheric Research</s1>
<s2>Boulder, Colorado</s2>
<s3>USA</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
<sZ>3 aut.</sZ>
<sZ>4 aut.</sZ>
<sZ>5 aut.</sZ>
<sZ>6 aut.</sZ>
<sZ>7 aut.</sZ>
</inist:fA14>
</affiliation>
</author>
<author><name sortKey="Walters, S" sort="Walters, S" uniqKey="Walters S" first="S." last="Walters">S. Walters</name>
<affiliation><inist:fA14 i1="01"><s1>National Center for Atmospheric Research</s1>
<s2>Boulder, Colorado</s2>
<s3>USA</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
<sZ>3 aut.</sZ>
<sZ>4 aut.</sZ>
<sZ>5 aut.</sZ>
<sZ>6 aut.</sZ>
<sZ>7 aut.</sZ>
</inist:fA14>
</affiliation>
</author>
<author><name sortKey="Guenther, A" sort="Guenther, A" uniqKey="Guenther A" first="A." last="Guenther">A. Guenther</name>
<affiliation><inist:fA14 i1="01"><s1>National Center for Atmospheric Research</s1>
<s2>Boulder, Colorado</s2>
<s3>USA</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
<sZ>3 aut.</sZ>
<sZ>4 aut.</sZ>
<sZ>5 aut.</sZ>
<sZ>6 aut.</sZ>
<sZ>7 aut.</sZ>
</inist:fA14>
</affiliation>
</author>
<author><name sortKey="Palmer, P I" sort="Palmer, P I" uniqKey="Palmer P" first="P. I." last="Palmer">P. I. Palmer</name>
<affiliation><inist:fA14 i1="02"><s1>School of GeoSciences, University of Edinburgh</s1>
<s2>Edinburgh</s2>
<s3>GBR</s3>
<sZ>8 aut.</sZ>
</inist:fA14>
</affiliation>
</author>
<author><name sortKey="Lawrence, P J" sort="Lawrence, P J" uniqKey="Lawrence P" first="P. J." last="Lawrence">P. J. Lawrence</name>
<affiliation><inist:fA14 i1="03"><s1>Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado</s1>
<s2>Boulder, Colorado</s2>
<s3>USA</s3>
<sZ>9 aut.</sZ>
</inist:fA14>
</affiliation>
</author>
</analytic>
<series><title level="j" type="main">Journal of geophysical research</title>
<title level="j" type="abbreviated">J. geophys. res.</title>
<idno type="ISSN">0148-0227</idno>
<imprint><date when="2008">2008</date>
</imprint>
</series>
</biblStruct>
</sourceDesc>
<seriesStmt><title level="j" type="main">Journal of geophysical research</title>
<title level="j" type="abbreviated">J. geophys. res.</title>
<idno type="ISSN">0148-0227</idno>
</seriesStmt>
</fileDesc>
<profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Carbon monoxide</term>
<term>Formaldehyde</term>
<term>Isoprene</term>
<term>Pan</term>
<term>Peroxyacetyl nitrate</term>
<term>Planetary scale</term>
<term>Trace compound</term>
<term>aerosols</term>
<term>carbon</term>
<term>carbon monoxide</term>
<term>concentration</term>
<term>gases</term>
<term>global</term>
<term>land cover</term>
<term>models</term>
<term>oxidation</term>
<term>ozone</term>
<term>sensitivity analysis</term>
<term>tracers</term>
<term>trajectory</term>
<term>transport</term>
<term>troposphere</term>
<term>variability</term>
</keywords>
<keywords scheme="Pascal" xml:lang="fr"><term>Isoprène</term>
<term>Modèle</term>
<term>Traceur</term>
<term>Analyse sensibilité</term>
<term>Monde</term>
<term>Transport</term>
<term>Occupation sol</term>
<term>Troposphère</term>
<term>Ozone</term>
<term>Gaz</term>
<term>Aérosol</term>
<term>Trajectoire</term>
<term>Carbone</term>
<term>Oxydation</term>
<term>Monoxyde carbone</term>
<term>Monoxyde de carbone</term>
<term>Formaldéhyde</term>
<term>Peracétique acide nitrate</term>
<term>Pan</term>
<term>Echelle planétaire</term>
<term>Concentration</term>
<term>Composé trace</term>
<term>Variabilité</term>
</keywords>
</textClass>
</profileDesc>
</teiHeader>
<front><div type="abstract" xml:lang="en">[1] We present a study of the sensitivity of isoprene emission calculations in a global chemistry transport model (CTM) to input land cover characteristics and analyze the impacts of changes in isoprene on the tropospheric budgets of atmospheric key species. The CTM Model for Ozone and Related Chemical Species, version 4 (MOZART-4) includes the online calculation of isoprene emissions based on the Model of Emissions of Gases and Aerosols from Nature (MEGAN), which is driven by three different land parameter inputs. We also included a tagging scheme in the CTM, which keeps track of the production of carbon containing species from isoprene oxidation. It is found that the amount of tropospheric carbon monoxide (CO), formaldehyde (HCHO) and peroxyacetylnitrate (PAN) explained by isoprene oxidation ranges from 9-16%, 15-27%, and 22-32%, depending on the isoprene emissions scenario. Changes in the global tropospheric burden with different land cover inputs can reach up to 10% for CO, 15% for HCHO, and 20% for PAN. Changes for ozone are small on a global scale, but regionally differences are as large as 3DU in the tropospheric column and as large as 5 ppbv in the surface concentrations. Our results demonstrate that a careful integration of isoprene emissions and chemistry in CTMs is very important for simulating the budgets of a number of atmospheric trace gases. We further demonstrate that the model tagging scheme has the capability of improving conventional methods of constraining isoprene emissions from space-borne HCHO column observations, especially in regions where a considerable part of the variability in the HCHO column is not related to isoprene.</div>
</front>
</TEI>
<inist><standard h6="B"><pA><fA01 i1="01" i2="1"><s0>0148-0227</s0>
</fA01>
<fA03 i2="1"><s0>J. geophys. res.</s0>
</fA03>
<fA05><s2>113</s2>
</fA05>
<fA06><s2>D5</s2>
</fA06>
<fA08 i1="01" i2="1" l="ENG"><s1>Contribution of isoprene to chemical budgets : A model tracer study with the NCAR CTM MOZART-4</s1>
</fA08>
<fA11 i1="01" i2="1"><s1>PFISTER (G. G.)</s1>
</fA11>
<fA11 i1="02" i2="1"><s1>EMMONS (L. K.)</s1>
</fA11>
<fA11 i1="03" i2="1"><s1>HESS (P. G.)</s1>
</fA11>
<fA11 i1="04" i2="1"><s1>LAMARQUE (J.-F.)</s1>
</fA11>
<fA11 i1="05" i2="1"><s1>ORLANDO (J. J.)</s1>
</fA11>
<fA11 i1="06" i2="1"><s1>WALTERS (S.)</s1>
</fA11>
<fA11 i1="07" i2="1"><s1>GUENTHER (A.)</s1>
</fA11>
<fA11 i1="08" i2="1"><s1>PALMER (P. I.)</s1>
</fA11>
<fA11 i1="09" i2="1"><s1>LAWRENCE (P. J.)</s1>
</fA11>
<fA14 i1="01"><s1>National Center for Atmospheric Research</s1>
<s2>Boulder, Colorado</s2>
<s3>USA</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
<sZ>3 aut.</sZ>
<sZ>4 aut.</sZ>
<sZ>5 aut.</sZ>
<sZ>6 aut.</sZ>
<sZ>7 aut.</sZ>
</fA14>
<fA14 i1="02"><s1>School of GeoSciences, University of Edinburgh</s1>
<s2>Edinburgh</s2>
<s3>GBR</s3>
<sZ>8 aut.</sZ>
</fA14>
<fA14 i1="03"><s1>Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado</s1>
<s2>Boulder, Colorado</s2>
<s3>USA</s3>
<sZ>9 aut.</sZ>
</fA14>
<fA20><s2>D05308.1-D05308.21</s2>
</fA20>
<fA21><s1>2008</s1>
</fA21>
<fA23 i1="01"><s0>ENG</s0>
</fA23>
<fA43 i1="01"><s1>INIST</s1>
<s2>3144</s2>
<s5>354000183022170370</s5>
</fA43>
<fA44><s0>0000</s0>
<s1>© 2008 INIST-CNRS. All rights reserved.</s1>
</fA44>
<fA45><s0>1 p.1/2</s0>
</fA45>
<fA47 i1="01" i2="1"><s0>08-0208587</s0>
</fA47>
<fA60><s1>P</s1>
</fA60>
<fA61><s0>A</s0>
</fA61>
<fA64 i1="01" i2="1"><s0>Journal of geophysical research</s0>
</fA64>
<fA66 i1="01"><s0>USA</s0>
</fA66>
<fC01 i1="01" l="ENG"><s0>[1] We present a study of the sensitivity of isoprene emission calculations in a global chemistry transport model (CTM) to input land cover characteristics and analyze the impacts of changes in isoprene on the tropospheric budgets of atmospheric key species. The CTM Model for Ozone and Related Chemical Species, version 4 (MOZART-4) includes the online calculation of isoprene emissions based on the Model of Emissions of Gases and Aerosols from Nature (MEGAN), which is driven by three different land parameter inputs. We also included a tagging scheme in the CTM, which keeps track of the production of carbon containing species from isoprene oxidation. It is found that the amount of tropospheric carbon monoxide (CO), formaldehyde (HCHO) and peroxyacetylnitrate (PAN) explained by isoprene oxidation ranges from 9-16%, 15-27%, and 22-32%, depending on the isoprene emissions scenario. Changes in the global tropospheric burden with different land cover inputs can reach up to 10% for CO, 15% for HCHO, and 20% for PAN. Changes for ozone are small on a global scale, but regionally differences are as large as 3DU in the tropospheric column and as large as 5 ppbv in the surface concentrations. Our results demonstrate that a careful integration of isoprene emissions and chemistry in CTMs is very important for simulating the budgets of a number of atmospheric trace gases. We further demonstrate that the model tagging scheme has the capability of improving conventional methods of constraining isoprene emissions from space-borne HCHO column observations, especially in regions where a considerable part of the variability in the HCHO column is not related to isoprene.</s0>
</fC01>
<fC02 i1="01" i2="3"><s0>001E</s0>
</fC02>
<fC02 i1="02" i2="2"><s0>001E01</s0>
</fC02>
<fC02 i1="03" i2="2"><s0>220</s0>
</fC02>
<fC03 i1="01" i2="X" l="FRE"><s0>Isoprène</s0>
<s2>NK</s2>
<s5>01</s5>
</fC03>
<fC03 i1="01" i2="X" l="ENG"><s0>Isoprene</s0>
<s2>NK</s2>
<s5>01</s5>
</fC03>
<fC03 i1="01" i2="X" l="SPA"><s0>Isopreno</s0>
<s2>NK</s2>
<s5>01</s5>
</fC03>
<fC03 i1="02" i2="2" l="FRE"><s0>Modèle</s0>
<s5>02</s5>
</fC03>
<fC03 i1="02" i2="2" l="ENG"><s0>models</s0>
<s5>02</s5>
</fC03>
<fC03 i1="02" i2="2" l="SPA"><s0>Modelo</s0>
<s5>02</s5>
</fC03>
<fC03 i1="03" i2="2" l="FRE"><s0>Traceur</s0>
<s5>03</s5>
</fC03>
<fC03 i1="03" i2="2" l="ENG"><s0>tracers</s0>
<s5>03</s5>
</fC03>
<fC03 i1="03" i2="2" l="SPA"><s0>Trazador</s0>
<s5>03</s5>
</fC03>
<fC03 i1="04" i2="2" l="FRE"><s0>Analyse sensibilité</s0>
<s5>04</s5>
</fC03>
<fC03 i1="04" i2="2" l="ENG"><s0>sensitivity analysis</s0>
<s5>04</s5>
</fC03>
<fC03 i1="05" i2="2" l="FRE"><s0>Monde</s0>
<s5>05</s5>
</fC03>
<fC03 i1="05" i2="2" l="ENG"><s0>global</s0>
<s5>05</s5>
</fC03>
<fC03 i1="05" i2="2" l="SPA"><s0>Mundo</s0>
<s5>05</s5>
</fC03>
<fC03 i1="06" i2="2" l="FRE"><s0>Transport</s0>
<s5>06</s5>
</fC03>
<fC03 i1="06" i2="2" l="ENG"><s0>transport</s0>
<s5>06</s5>
</fC03>
<fC03 i1="06" i2="2" l="SPA"><s0>Transporte</s0>
<s5>06</s5>
</fC03>
<fC03 i1="07" i2="2" l="FRE"><s0>Occupation sol</s0>
<s5>07</s5>
</fC03>
<fC03 i1="07" i2="2" l="ENG"><s0>land cover</s0>
<s5>07</s5>
</fC03>
<fC03 i1="08" i2="2" l="FRE"><s0>Troposphère</s0>
<s5>08</s5>
</fC03>
<fC03 i1="08" i2="2" l="ENG"><s0>troposphere</s0>
<s5>08</s5>
</fC03>
<fC03 i1="09" i2="2" l="FRE"><s0>Ozone</s0>
<s5>09</s5>
</fC03>
<fC03 i1="09" i2="2" l="ENG"><s0>ozone</s0>
<s5>09</s5>
</fC03>
<fC03 i1="09" i2="2" l="SPA"><s0>Ozono</s0>
<s5>09</s5>
</fC03>
<fC03 i1="10" i2="2" l="FRE"><s0>Gaz</s0>
<s5>10</s5>
</fC03>
<fC03 i1="10" i2="2" l="ENG"><s0>gases</s0>
<s5>10</s5>
</fC03>
<fC03 i1="10" i2="2" l="SPA"><s0>Gas</s0>
<s5>10</s5>
</fC03>
<fC03 i1="11" i2="2" l="FRE"><s0>Aérosol</s0>
<s5>11</s5>
</fC03>
<fC03 i1="11" i2="2" l="ENG"><s0>aerosols</s0>
<s5>11</s5>
</fC03>
<fC03 i1="11" i2="2" l="SPA"><s0>Aerosol</s0>
<s5>11</s5>
</fC03>
<fC03 i1="12" i2="2" l="FRE"><s0>Trajectoire</s0>
<s5>12</s5>
</fC03>
<fC03 i1="12" i2="2" l="ENG"><s0>trajectory</s0>
<s5>12</s5>
</fC03>
<fC03 i1="13" i2="2" l="FRE"><s0>Carbone</s0>
<s5>13</s5>
</fC03>
<fC03 i1="13" i2="2" l="ENG"><s0>carbon</s0>
<s5>13</s5>
</fC03>
<fC03 i1="13" i2="2" l="SPA"><s0>Carbono</s0>
<s5>13</s5>
</fC03>
<fC03 i1="14" i2="2" l="FRE"><s0>Oxydation</s0>
<s5>14</s5>
</fC03>
<fC03 i1="14" i2="2" l="ENG"><s0>oxidation</s0>
<s5>14</s5>
</fC03>
<fC03 i1="14" i2="2" l="SPA"><s0>Oxidación</s0>
<s5>14</s5>
</fC03>
<fC03 i1="15" i2="2" l="FRE"><s0>Monoxyde carbone</s0>
<s5>15</s5>
</fC03>
<fC03 i1="15" i2="2" l="ENG"><s0>carbon monoxide</s0>
<s5>15</s5>
</fC03>
<fC03 i1="16" i2="X" l="FRE"><s0>Monoxyde de carbone</s0>
<s2>NK</s2>
<s2>FX</s2>
<s5>16</s5>
</fC03>
<fC03 i1="16" i2="X" l="ENG"><s0>Carbon monoxide</s0>
<s2>NK</s2>
<s2>FX</s2>
<s5>16</s5>
</fC03>
<fC03 i1="16" i2="X" l="SPA"><s0>Carbono monóxido</s0>
<s2>NK</s2>
<s2>FX</s2>
<s5>16</s5>
</fC03>
<fC03 i1="17" i2="X" l="FRE"><s0>Formaldéhyde</s0>
<s2>NK</s2>
<s2>FX</s2>
<s5>17</s5>
</fC03>
<fC03 i1="17" i2="X" l="ENG"><s0>Formaldehyde</s0>
<s2>NK</s2>
<s2>FX</s2>
<s5>17</s5>
</fC03>
<fC03 i1="17" i2="X" l="SPA"><s0>Formaldehído</s0>
<s2>NK</s2>
<s2>FX</s2>
<s5>17</s5>
</fC03>
<fC03 i1="18" i2="3" l="FRE"><s0>Peracétique acide nitrate</s0>
<s2>NK</s2>
<s5>18</s5>
</fC03>
<fC03 i1="18" i2="3" l="ENG"><s0>Peroxyacetyl nitrate</s0>
<s2>NK</s2>
<s5>18</s5>
</fC03>
<fC03 i1="19" i2="X" l="FRE"><s0>Pan</s0>
<s2>NO</s2>
<s5>19</s5>
</fC03>
<fC03 i1="19" i2="X" l="ENG"><s0>Pan</s0>
<s2>NO</s2>
<s5>19</s5>
</fC03>
<fC03 i1="19" i2="X" l="SPA"><s0>Pan</s0>
<s2>NO</s2>
<s5>19</s5>
</fC03>
<fC03 i1="20" i2="X" l="FRE"><s0>Echelle planétaire</s0>
<s5>20</s5>
</fC03>
<fC03 i1="20" i2="X" l="ENG"><s0>Planetary scale</s0>
<s5>20</s5>
</fC03>
<fC03 i1="20" i2="X" l="SPA"><s0>Escala planetaria</s0>
<s5>20</s5>
</fC03>
<fC03 i1="21" i2="2" l="FRE"><s0>Concentration</s0>
<s5>21</s5>
</fC03>
<fC03 i1="21" i2="2" l="ENG"><s0>concentration</s0>
<s5>21</s5>
</fC03>
<fC03 i1="21" i2="2" l="SPA"><s0>Concentración</s0>
<s5>21</s5>
</fC03>
<fC03 i1="22" i2="X" l="FRE"><s0>Composé trace</s0>
<s5>22</s5>
</fC03>
<fC03 i1="22" i2="X" l="ENG"><s0>Trace compound</s0>
<s5>22</s5>
</fC03>
<fC03 i1="22" i2="X" l="SPA"><s0>Compuesto huella</s0>
<s5>22</s5>
</fC03>
<fC03 i1="23" i2="2" l="FRE"><s0>Variabilité</s0>
<s5>23</s5>
</fC03>
<fC03 i1="23" i2="2" l="ENG"><s0>variability</s0>
<s5>23</s5>
</fC03>
<fN21><s1>133</s1>
</fN21>
<fN44 i1="01"><s1>OTO</s1>
</fN44>
<fN82><s1>OTO</s1>
</fN82>
</pA>
</standard>
<server><NO>PASCAL 08-0208587 INIST</NO>
<ET>Contribution of isoprene to chemical budgets : A model tracer study with the NCAR CTM MOZART-4</ET>
<AU>PFISTER (G. G.); EMMONS (L. K.); HESS (P. G.); LAMARQUE (J.-F.); ORLANDO (J. J.); WALTERS (S.); GUENTHER (A.); PALMER (P. I.); LAWRENCE (P. J.)</AU>
<AF>National Center for Atmospheric Research/Boulder, Colorado/Etats-Unis (1 aut., 2 aut., 3 aut., 4 aut., 5 aut., 6 aut., 7 aut.); School of GeoSciences, University of Edinburgh/Edinburgh/Royaume-Uni (8 aut.); Cooperative Institute for Research in Environmental Sciences (CIRES), University of Colorado/Boulder, Colorado/Etats-Unis (9 aut.)</AF>
<DT>Publication en série; Niveau analytique</DT>
<SO>Journal of geophysical research; ISSN 0148-0227; Etats-Unis; Da. 2008; Vol. 113; No. D5; D05308.1-D05308.21; Bibl. 1 p.1/2</SO>
<LA>Anglais</LA>
<EA>[1] We present a study of the sensitivity of isoprene emission calculations in a global chemistry transport model (CTM) to input land cover characteristics and analyze the impacts of changes in isoprene on the tropospheric budgets of atmospheric key species. The CTM Model for Ozone and Related Chemical Species, version 4 (MOZART-4) includes the online calculation of isoprene emissions based on the Model of Emissions of Gases and Aerosols from Nature (MEGAN), which is driven by three different land parameter inputs. We also included a tagging scheme in the CTM, which keeps track of the production of carbon containing species from isoprene oxidation. It is found that the amount of tropospheric carbon monoxide (CO), formaldehyde (HCHO) and peroxyacetylnitrate (PAN) explained by isoprene oxidation ranges from 9-16%, 15-27%, and 22-32%, depending on the isoprene emissions scenario. Changes in the global tropospheric burden with different land cover inputs can reach up to 10% for CO, 15% for HCHO, and 20% for PAN. Changes for ozone are small on a global scale, but regionally differences are as large as 3DU in the tropospheric column and as large as 5 ppbv in the surface concentrations. Our results demonstrate that a careful integration of isoprene emissions and chemistry in CTMs is very important for simulating the budgets of a number of atmospheric trace gases. We further demonstrate that the model tagging scheme has the capability of improving conventional methods of constraining isoprene emissions from space-borne HCHO column observations, especially in regions where a considerable part of the variability in the HCHO column is not related to isoprene.</EA>
<CC>001E; 001E01; 220</CC>
<FD>Isoprène; Modèle; Traceur; Analyse sensibilité; Monde; Transport; Occupation sol; Troposphère; Ozone; Gaz; Aérosol; Trajectoire; Carbone; Oxydation; Monoxyde carbone; Monoxyde de carbone; Formaldéhyde; Peracétique acide nitrate; Pan; Echelle planétaire; Concentration; Composé trace; Variabilité</FD>
<ED>Isoprene; models; tracers; sensitivity analysis; global; transport; land cover; troposphere; ozone; gases; aerosols; trajectory; carbon; oxidation; carbon monoxide; Carbon monoxide; Formaldehyde; Peroxyacetyl nitrate; Pan; Planetary scale; concentration; Trace compound; variability</ED>
<SD>Isopreno; Modelo; Trazador; Mundo; Transporte; Ozono; Gas; Aerosol; Carbono; Oxidación; Carbono monóxido; Formaldehído; Pan; Escala planetaria; Concentración; Compuesto huella</SD>
<LO>INIST-3144.354000183022170370</LO>
<ID>08-0208587</ID>
</server>
</inist>
</record>

Pour manipuler ce document sous Unix (Dilib)

EXPLOR_STEP=$WICRI_ROOT/Wicri/Musique/explor/MozartV1/Data/PascalFrancis/Corpus

HfdSelect -h $EXPLOR_STEP/biblio.hfd -nk 000112 | SxmlIndent | more

HfdSelect -h $EXPLOR_AREA/Data/PascalFrancis/Corpus/biblio.hfd -nk 000112 | SxmlIndent | more

Pour mettre un lien sur cette page dans le réseau Wicri

{{Explor lien
   |wiki=    Wicri/Musique
   |area=    MozartV1
   |flux=    PascalFrancis
   |étape=   Corpus
   |type=    RBID
   |clé=     Pascal:08-0208587
   |texte=   Contribution of isoprene to chemical budgets : A model tracer study with the NCAR CTM MOZART-4
}}

This area was generated with Dilib version V0.6.20.
Data generation: Sun Apr 10 15:06:14 2016. Site generation: Tue Feb 7 15:40:35 2023

	Serveur d'exploration sur Mozart
	Attention, ce site est en cours de développement ! Attention, site généré par des moyens informatiques à partir de corpus bruts. Les informations ne sont donc pas validées.

Serveur d'exploration sur Mozart

Contribution of isoprene to chemical budgets : A model tracer study with the NCAR CTM MOZART-4

Contribution of isoprene to chemical budgets : A model tracer study with the NCAR CTM MOZART-4

Source :

Descripteurs français

English descriptors

Abstract

Notice en format standard (ISO 2709)

Format Inist (serveur)

Links to Exploration step

Le document en format XML

Pour manipuler ce document sous Unix (Dilib)

Pour mettre un lien sur cette page dans le réseau Wicri